A novel ultrafast multiple-mode multiple-dimensional vibrational spectroscopic method was constructed based on a super broadband IR/THz pusle, using the ps/fs hybridization scheme. We were able to determine 3D molecular comfornations and structures with the method. Its principles and applications in determining molecular structures in liquids, regular crystals, plastic crystals, glass, and on the surfaces of nanomaterials will be introduced.

Super IR-continuum-based multiple-mode multiple-dimensional vibrational spectroscopy

245th National Meeting (2013)

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