Porous organic polymers (POPs) are a class of amorphous porous polymers that are composed of light elements (C, H, O, N, and B) linked via strong covalent bonds. POPs are generally constructed by using reversible or irreversible bond forming reactions to yield porous polymers high surface areas, high chemical, and high thermal stabilities. These features make POPs useful for carbon capture, gas storage, and catalytic applications. This lecture will discuss employing a bottom-up approach to create metalated POPs for the hydrosilylative reduction of CO2 to potassium formate and methanol. The prospect of using metalated POPs to capture and convert CO2 to an alternative fuel source will be highlighted.

Metalated porous organic polymers for the hydrosilylative reduction of CO2 to formate and methanol

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ACS Fall 2022

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