The preparation of large-sized single crystals of two-dimensional polymer (2DP) frameworks is a big challenge and significantly important. The successful examples are extremely rare. Considering the difficulty and importance in preparing large-size single-crystal 2DP frameworks, we try to realize the preparation of large-size single crystals of 2DP materials through a single-crystal-to-single-crystal strategy. The orientation of the arrangement and stacking mode will be realized during the crystallization process. The long-range ordered structure can greatly improve the electronic performance of the material. Precise pores with atomic resolution will promote the application of 2DP in the field of electronic devices and separation membrane materials.

Large-sized single crystals of two-dimensional polymer frameworks

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